ains Malaysiana 52(7)(2023): 2095-2102
http://doi.org/10.17576/jsm-2023-5207-15
Anomali Halaju Bunyi Ricih dan Atenuasi Ultrasonik
dalam TmBa2Cu3O7-d (d = 0.06 dan 0.6)
(Shear Sound Velocity and Ultrasonic Attenuation
Anomalies in TmBa2Cu3O7-d (d = 0.06 and 0.6))
R. ABD-SHUKOR1,*, B.B.
LEE1, K. MUHAMMAD-NAJIB1, NOR AZAH NIK-JAAFAR2 & MOHD NARIZEE MOHD NASIR1
1Department of Applied Physics,
Universiti Kebangsaan Malaysia, 43600 Bangi, Selangor, Malaysia
2Pusat PERMATA@Pintar Negara, Universiti Kebangsaan Malaysia, 43600 Bangi, Selangor, Malaysia
Received: 15 May
2023/Accepted: 3 July 2023
Abstrak
Halaju bunyi,
dan atenuasi ultrasonik, a gelombang ricih dalam
TmBa2Cu3O6.94 yang mensuperkonduksi dan TmBa2Cu3O6.40 yang tidak mensuperkonduksi telah diukur daripada 80 dan 200 K pada julat
frekuensi MHz. Sampel superkonduktor TmBa2Cu3O6.94 menunjukkan
histeresis terma dan peningkatan halaju ricih,
sebanyak 2.5% apabila suhu diturunkan
daripada 200 K hingga 80 K. Sampel TmBa2Cu3O6.40 yang bukan superkonduktor pula menunjukkan
peningkatan
= 1.5% apabila suhu
diturunkan dalam julat suhu yang sama. Tiada histerisis yang ketara dicerap dalam sampel TmBa2Cu3O6.40 yang bukan superkonduktor. Superkonduktor TmBa2Cu3O6.94 menunjukkan halaju bunyi ricih meningkat dengan ketara berhampiran suhu
genting mula (Tc-mula = 93 K) semasa penyejukan tetapi tidak
semasa pemanasan. Sampel superkonduktor TmBa2Cu3O6.94 juga menunjukkan puncak atenuasi berhampiran suhu genting. Di samping itu wujud puncak atenuasi yang
lebar pada 140 K semasa suhu menaik dan 160 K semasa suhu menurun bagi sampel
TmBa2Cu3O6.94 yang mensuperkonduksi. Anomali ultrasonik dalam superkonduktor TmBa2Cu3O6.94 diterangkan menggunakan
kandungan oksigen dan tertiban oksigen dalam satah dan rantai kuprum oksida.
Kata kunci: Halaju bunyi; modulus ricih;
pembelauan sinar-X; tertiban oksigen
Abstract
Sound velocity,
and ultrasonic
attenuation, a of shear waves in superconducting TmBa2Cu3O6.94 and non-superconducting TmBa2Cu3O6.40 were
measured from 80 to 200 K in the MHz frequency range. The superconducting TmBa2Cu3O6.94 showed a thermal hysteresis and increased shear velocity,
by 2.5% when the temperature was lowered from
200 K to 80 K. The non-superconducting sample TmBa2Cu3O6.40 showed an increase in the shear velocity,
by 1.5% when the temperature was lowered in
the same range. No significant
hysteresis was observed in the non-superconducting TmBa2Cu3O6.40.
The superconducting TmBa2Cu3O6.94 showed a
significant increase in the shear velocity near the onset critical temperature
(Tc-onset = 93 K) during cooling but not warming. The
superconducting sample TmBa2Cu3O6.94 also
showed an attenuation peak near the critical temperature. In addition, a broad
attenuation peak was observed at 140 K during warming and 160 K during cooling
for the superconducting TmBa2Cu3O6.94 sample.
The ultrasonic anomalies observed in the superconducting TmBa2Cu3O6.94 was explained in terms of oxygen content and oxygen orderings in the copper
oxide chains and layers.
Keywords: Oxygen orderings; shear modulus; sound
velocity; X-ray diffraction
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*Corresponding author; email:
ras@ukm.edu.my
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